Machine Olfaction Device (MOD) Sensors (Part One)

There are a number of different types of sensors(SnO2). This is later ground and mixed with dopands
which can be used as essential components in(usually metal chlorides) and then heated to recover
different designs for machine olfaction systems.the pure metal as a powder.
1. Electrochemical sensors.For the purpose of screen printing, a paste is made
2. Metal oxide semiconductors.up from the powder.
3. Schottky diode-based sensors.Finally, in a layer of few hundred microns, the paste
4. Calorimetric sensors.will be left to cool (e.g. on a alumina tube or plain
5. Quartz crystal microbalances.substrate).b. Sensing Mechanism
6. Optical sensors.Change of "conductance" in the MOS is the basic
Electronic Nose (or eNose) sensors fall into fiveprinciple of the operation in the sensor itself. A
categories [1]: conductivity sensors, piezoelectricchange in conductance takes place when an
sensors, Metal Oxide Field Effect Transistorsinteraction with a gas happens, the conductance
(MOSFETs), optical sensors, and these employingvarying depending on the concentration of the gas
spectrometry-based sensing methods.itself.
Conductivity sensors may be composed of metalMetal oxide sensors fall into two types [2]:
oxide and polymer elements, both of which exhibit a
change in resistance when exposed to Volatile1. n-type (zinc oxide (ZnO), tin dioxide (SnO2),
Organic Compounds (VOCs) [1].titanium dioxide (TiO2) iron (III) oxide (Fe2O3).
In this report only Metal Oxide Semi-conductor2. p-type (nickel oxide (Ni2O3), cobalt oxide (CoO).
(MOS), Conducting Polymer (CP) and Quartz CrystalThe n type usually responds to "reducing" gases,
Microbalance (QCM) will be examined, as they arewhile the p-type responds to "oxidizing" vapours.
well researched, documented and established asOperation (n-type) [2]:
important element for various types of machineAs the current applied between the two electrodes,
olfaction devices. The application, where thevia "the metal oxide", oxygen in the air start to react
proposed device will be trained on to analyse, willwith the surface and accumulate on the surface of
greatly influence the choice of sensor.the sensor, consequently "trapping free electrons on
The response of the sensor is a two part processthe surface from the conduction band" [2]. In this
[3]:way, the electrical conductance decreases as
resistance in these areas increase due to lack of
1. The vapour pressure of the analyte usually dictatescarriers (i.e. increase resistance to current), as there
how many molecules are present in the gas phasewill be a "potential barriers" between the grains
and consequently how many of them will be at the(particles) themselves.
sensor(s).When the sensor exposed to reducing gases (e.g.
2. When the gas-phase molecules are at theCO) then the resistance drop, as the gas usually
sensor(s), these molecules need to be able to reactreact with the oxygen and therefore, an electron will
with the sensor(s) in order to produce a response.be released. Consequently, the release of the
Sensors types used in any machine olfaction deviceelectron increase the conductivity as it will reduce
can be mass transducers e.g. QMB "Quartz"the potential barriers" and let the electrons to start
microbalance" or chemoresistors i.e. based on metal-to flow [2].
oxide or conducting polymers. In some cases, arraysOperation (p-type):
may contain both of the above two types ofOxidising gases (e.g. O2, NO2) usually remove
sensors [4].electrons from the surface of the sensor, and
Metal-Oxide Semiconductorsconsequently, as a result of this charge carriers will
These sensors were originally produced in Japan inbe produced.c. Limitation of MOS sensors [4]
the 1960s and used in "gas alarm" devices.1. Poor Selectivity - In particular when a thick film
Metal oxide semiconductors (MOS) have been usedMOS device is used. The poor selectivity can be
more extensively in electronic nose instruments andreduced by the deposition of a suitable catalyst layer
are widely available commercially [1].of noble metals like Pd, Pt, Au and Ag.
MOS are made of a ceramic element heated by a2. MOS need high temperatures (around 300°c)
heating wire and coated by a semiconducting film.to operate efficiently; this result higher power
They can sense gases by monitoring changes in theconsumption.
conductance during the interaction of a chemically3. Sensitive to humidity and to compounds such as
sensitive material with molecules that need to beethanol and CO2.d. Advantages [4]
detected in the gas phase. Out of many MOS, the1. Widely available in a variety of types and
material which has been experimented with the mostsensitivities.
is tin dioxide (SnO2) - this is because of its stability2. Very sensitive to a number of organic vapours (e.g.
and sensitivity at lower temperatures. Differentoil).
types of MOS may include oxides of tin, zinc,3. Fast response, usually less than 10 seconds.
titanium, tungsten, and iridium, doped with a nobleAltawell
metal catalyst such as platinum or palladium.© Altawell 2008
MOS are subdivided into two types [4]: Thick FilmReferences
and Thin Film[1] Nagle, H. T., Schiffman, S. S., Gutierrez-Osuna,
Limitation of Thick Film MOS: Less sensitive (poorR.(1998) "The How and Why of
selectivity), it require a longer time to stabilize, higherElectronic Noses" IEEE Spectrum September 1998,
power consumption. This type of MOS is easier toVolume 35, Number 9, pp. 22-34.
produce and therefore, cost less to purchase.[2] Arshak K., Moore E., Lyons G.M., Harris J., Clifford
Limitation of Thin Film MOS: unstable, difficult toS "A review of gassensors employed in
produce and therefore, more expensive to purchase.electronicnose applications". (2004).
On the other hand, it has much higher sensitivity, and[3] Hurst, W. J., (1999) "Electronic Noses &
much lower power consumption than the thick filmSensory Array Based Systems".
MOS device [5].a. Manufacturing process [5]Technomic Publishing Company, ISBN No.
Polycrystalline is the most common porous material1-56676-780-6.
used for thick film sensors. It is usually prepared in a[4] Sberveglieri D., (1999) "Metal-Oxide
"sol-gel" process [5]:Semicondictors" ASTEQ Technologies for sensors
Tin tetrachloride (SnCl4) is prepared in an aqueous1999
solution, to which is added ammonia (NH3). This[5] Nose Office (2003) "NOSE II - The Second
precipitates tin tetra hydroxide which is dried andNetwork on Artificial Olfactory Sensing".
calcined at 500 - 1000°C to produce tin dioxide